I find the big benefit of Altair is that the API is so nice and composable, and because vega provides a ton out of the box to build really high quality visualisations.
It's also great being able to add Altair shapes to Folium for geoplotting (as the vega geoplotting is a bit more low-level).
What I really think is missing in the ecosystem is a "vega for tables", so you could be rich, interactive tables with a similar grammar. That would rock.
It helped me settle on https://altair-viz.github.io/ (coming from matplotlib) and I never looked back